Designing New Functional Materials at the Atomic Scale
News and Cover Articles
News: https://newscenter.lbl.gov/2019/04/18/electric-skyrmions-charge-ahead-for-next-generation-data-storage/
Youtube Video: https://www.youtube.com/watch?v=Lhx37IssMCw
Physical Review Lett. 129, 247601 (2022)
Nature 592, 376-380 (2021)
Nature Materials 18, 377-383 (2019)
Advanced Materials 36, 2405294 (2024)
Link: https://phys.org/news/2024-10-material-pulses-energy-efficient-supercomputing.html
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Selected Publications:
($ corresponding author; * equally contributed author)
1. Observation of room temperature polar skyrmions
S. Das*$, Y. L. Tang*, Z. Hong*, M. A. P. Gonçalves*, M. R. McCarter, C. Klewe, K.X. Nyugen, F. Gómez-Ortiz, P. Shafer, E. Arenholz, V. A. Stoica, S.-L. Hsu, B. Wang, C. Ophus, J. F. Liu, C. T. Nelson, S. Saremi, B. Prasad, A. B. Mei, D. G. Schlom, J. Íñiguez, P. García-Fernández, D.A. Muller, L. Q. Chen, J. Junquera, L. W. Martin and R. Ramesh$
Nature 568, 368-372 (2019)
DOI: https://doi.org/10.1038/s41586-019-1092-8
2. Local negative permittivity and topological phase-transition in polar skyrmions
S. Das*$, Z. Hong*, V.A. Stoica*, M. A. P. Gonçalves*, Y.T. Shao, E. Parsonnet, E. J. Marksz, S. Saremi, M. R. McCarter, A. Reynoso, C. J Long, A. M. Hagerstrom, D. Meyers, V. Ravi, B. Prasad, H. Zhou, Z. Zhang, H. Wen, F. Gómez-Ortiz, P. García-Fernández, J. Bokor, J. Íñiguez, J.W. Freeland, N. D. Orloff, J. Junquera, L.Q. Chen, S. Salahuddin, D. A. Muller, L.W. Martin, R. Ramesh$
Nature Materials 20, 194-201 (2021)
DOI: https://doi.org/10.1038/s41563-020-00818-y
3. Metamorphosis of topological spin structures
Jayjit Kumar Dey, Sujit Das*
Nature Physics: News and Views (2024)
DOI: https://doi.org/10.1038/s41567-024-02514-z
4. Low voltage-driven high-performance thermal switching in antiferroelectric PbZrO3 thin films
Chenhan Liu, Yangyang Si, Hua Zhang, Chao Wu, Shiqing Deng, Yongqi Dong, Yijie Li, Meng Zhuo, Ningbo Fan, Bin Xu, Ping Lu, Lifa Zhang, Xi Lin, Xingjun Liu, Juekuan Yang, Zhenlin Luo, Sujit Das, Laurent Bellaiche, Yunfei Chen, Zuhuang Chen
Science 382, 1265-1269 (2023)
5. Emergent Chirality in a Polar Meron to Skyrmion Phase Transition
Yu-Tsun Shao, Sujit Das, Zijian Hong, Ruijuan Xu, Swathi Chandrika, Fernando Gómez- Ortiz, Pablo García-Fernández, Long-Qing Chen, Harold Y. Hwang, Javier Junquera, Lane W. Martin, Ramamoorthy Ramesh & David A. Muller
Nature Communications 14, 1355 (2023)
DOI: https://doi.org/10.1038/s41467-023-36950-x
6. Optical Control of Adaptive Nanoscale Domain Networks
Marc Zajac, Tao Zhou, Tiannan Yang, Sujit Das, Yue Cao, Burak Guzelturk, Vladimir Stoica, Mathew Cherukara, John W Freeland, Venkatraman Gopalan, Ramamoorthy Ramesh, Lane W Martin, Long-Qing Chen, Martin Holt, Stephan Hruszkewycz, Haidan Wen
Advanced Materials (2024)
7. Non-equilibrium pathways to emergent polar supertextures
Vladimir A Stoica*, Tiannan Yang*, Sujit Das*, Yue Cao, Huaiyu Wang, Yuya Kubota, Cheng Dai, Hari Padmanabhan, Yusuke Sato, Anudeep Mangu, Quynh L Nguyen, Zhan Zhang, Disha Talreja, Marc E Zajac, Donald A Walko, Anthony D DiChiara, Shigeki Owada, Kohei Miyanishi, Kenji Tamasaku, Takahiro Sato, James M Glownia, Vincent Esposito, Silke Nelson, Matthias C Hoffmann, Richard D Schaller, Aaron M Lindenberg, Lane W Martin, Ramamoorthy Ramesh, Iwao Matsuda, Diling Zhu, Long-Q Chen, Haidan Wen, Venkatraman Gopalan, John W Freeland
Nature Materials (2024)
8. Optical Creation of an Oxide Supercrystal with Three-Dimensional Nanoscale Periodicity
V.A. Stoica, N. Laanait, C. Dai, Z. Hong, Y. Yuan, Z. Zhang, S. Lei, M.R. McCarter, A. Yadav, A. R. Damodaran, S. Das, G.A. Stone, J. Karapetrova, D.A. Walko, X. Zhang, L. W. Martin, R. Ramesh, L.-Q. Chen, H. Wen, V. Gopalan, and J.W. Freeland
Nature Materials 18, 377-383 (2019)
DOI: https://doi.org/10.1038/s41563-019-0311-x
Cover article
9. Observation of Spatially Resolved Steady State Negative Capacitance
Ajay K. Yadav, Kayla X. Nguyen, Zijian Hong, Pablo García-Fernández, Pablo Aguado-Puente, Christopher T. Nelson, Sujit Das, Bhagwati Prasad, Daewoong Kwon, Suraj Cheema, Asif I. Khan, Jorge Íñiguez, Javier Junquera, Long-Qing Chen, David A. Muller, Ramamoorthy Ramesh, Sayeef Salahuddin
Nature 565, 468-471 (2019)
DOI: https://doi.org/10.1038/s41586-018-0855-y
10. Low-field switching of non-collinear spin textures at La0.7Sr0.3MnO3-SrRuO3 interfaces
S. Das$, A.D. Rata, I.V. Maznichenko, S. Agrestini, E. Pippel, K. Chen, E. Pellegrin, S. M. Valvidares, H. B. Vasili, J. Herrero-Martin, K. Nenkov, A. Herklotz, A. Ernst, I. Mertig, Z. Hu, and K. Dörr$
Phys. Rev. B 99, 024416 (2019)
DOI: https://doi.org/10.1103/PhysRevB.99.024416
11. Electric field manipulation of spins in doped PbTiO3
Junjie Liu, Valentin V. Laguta, Katherine Inzani, Weichuan Huang, Sujit Das, Ruchira Chatterjee, Evan Sheridan, Sinéad M. Griffin, Arzhang Ardavan, and Ramamoorthy Ramesh
Science Advances 7, eabf8103 (2021)
DOI: 10.1126/sciadv.abf8103
12. Inherent spin–polarization coupling in a magnetoelectric vortex
Sujit Das,*$ Valentyn Laguta,* Katherine Inzani,* Weichuan Huang, Junjie Liu, Ruchira Chatterjee, Margaret R. McCarter, Sandhya Susarla, Arzhang Ardavan, Javier Junquera, Sinéad M. Griffin, and Ramamoorthy Ramesh
Nano Letters 10, 3976-3982 (2022)
DOI: 10.1021/acs.nanolett.2c00496
13. Subterahertz collective dynamics of polar vortices
Qian Li*, Vladimir Stoica*, Marek Pasciak, Yi Zhu, Yakun Yuan, Tiannan Yang, Margaret R. McCarter, Sujit Das, Ajay K. Yadav, Suji Park, Cheng Dai, Hyeon Jun Lee, Youngjun Ahn, Samuel D. Marks, Takahiro Sato, Matthias C. Hoffmann, Matthieu Chollet, Michael E. Kozina, Silke Nelson, Diling Zhu, Donald A. Walko, Aaron M. Lindenberg, Paul G. Evans, Long-Qing Chen, R. Ramesh, Lane W. Martin, Venkatraman Gopalan, John W. Freeland, Jirka Hlinka, Haidan Wen
Nature 592, 376-380 (2021)
DOI: https://doi.org/10.1038/s41586-021-03342-4
14. Atomic scale crystal field mapping of the polar vortices in oxide superlattices
Sandhya Susarla, Colin Ophus, Pablo Garcia Fernandez, Sujit Das, Peter Ercius, Lane W. Martin, Ramamoorthy Ramesh and Javier Junquera.
Nature Communications 12, 6273 (2021)
DOI: https://doi.org/10.1038/s41467-021-26476-5
15. Vortex Domain Walls in Ferroelectrics
Z. Hong*, S. Das*, C. T. Nelson*, A. Yadav, Y. Wu, J. Junquera, L.-Q. Chen, L. W. Martin, R. Ramesh
Nano Letters 21, 3533-3539 (2021)
DOI: https://doi.org/10.1021/acs.nanolett.1c00404
16. Structural Chirality of Polar Skyrmions Probed by Resonant Elastic X-ray Scattering
Margaret R. McCarter,∗ Kook Tae Kim, ∗ Vladimir A. Stoica, Sujit Das, Christoph Klewe, Elizabeth P. Donoway, David M. Burn, Padraic Shafer, Fanny Rodolakis, Mauro A. P. Gonalves, Fernando G ́omez-Ortiz, Jorge Iniguez, Pablo Garcia-Fernandez, Javier Junquera, Stephen W. Lovesey, Gerrit van der Laan, Se Young Park, John W. Freeland, Lane W. Martin, Dong Ryeol Lee,$ and Ramamoorthy Ramesh$
Physical Review Lett. 129, 247601 (2022)
DOI: https://doi.org/10.1103/PhysRevLett.129.247601
17. Study of disorder in pulsed laser deposited double perovskite oxides by first-principle structure prediction
Edoardo Fertitta, Sujit Das, Debalina Banerjee, Farbod Ebrahimi, Clément Barraud, Kai Du, He Tian, Chris J. Pickard, Cedric Weber, Ramamoorthy Ramesh, Peter Littlewood, and David Dubbink
npj computational materials 7, 1-8 (2021)
DOI: https://doi.org/10.1038/s41524-021-00561-1
18. Epitaxial ferroelectric with metallic pyrochlore oxide electrodes
Z. Zhang, S.-L. Hsu, V. Stoica, H. Paik, J. Wang, L. Xie, M. Kumari, S. Das, Z. Leng, E.Parsonnet, A. Qualls, M. McBriarty, R. Proksch, A. Gruverman, D. G. Schlom, L.Q. Chen, S. Salahuddin, L. W. Martin, R. Ramesh
Advanced Materials 33, 2006089 (2021)
DOI: https://doi.org/10.1002/adma.202006089
19. Erbium-Implanted Materials for Quantum Communication Applications
Paul Stevenson, Christopher M Phenicie, Isaiah Gray, Sebastian P Horvath, Sacha Welinski, Austin M Ferrenti, Alban Ferrier, Philippe Goldner, Sujit Das, Ramamoorthy Ramesh, Robert J Cava, Nathalie P de Leon, and Jeff D Thompson
Physical Rev. B 105, 224116 (2022)
DOI: https://doi.org/10.1103/PhysRevB.105.224106
20. Strain dependence of the antiferromagnetic interface coupling in La0.7Sr0.3MnO3/SrRuO3 superlattice
Sujit Das$, Andreas Herklotz, Eckhard Pippel, Er-Jia Guo, Diana Rata and Kathrin Dörr$
Phys. Rev. B 91, 134405 (2015)
DOI: https://doi.org/10.1103/PhysRevB.91.134405
21. The role of lattice dynamics in ferroelectric switching
Qiwu Shi, Eric Parsonnet, Xiaoxing Chen, Ren-Ci Peng, Abel Fernandez, Natalya Fedorova, Alexander Qualls, Xiaoxi Huang, Xue Chang, Hongrui Zhang, David Pesquera, Sujit Das, Dmitri Nikonov, Ian Young, Long-Qing Chen, Lane Martin, Yen-Lin Huang, Jorge Íñiguez, Ramamoorthy Ramesh
Nature Communications 13, 1110 (2022)
DOI: https://doi.org/10.1038/s41467-022-28622-z
22. Room-temperature ferromagnetism at an oxide/nitride interface
Qiao Jin, Zhiwen Wang, Qinghua Zhang, Yonghong Yu, Shan Lin, Shengru Chen, Mingqun Qi, He Bai, Amanda Huon, Qian Li, Le Wang, Xinmao Yin, Chi Sin Tang, Andrew T. S. Wee, Fanqi Meng, Jiali Zhao, Jia-Ou Wang, Haizhong Guo, Chen Ge, Can Wang, Wensheng Yan, Tao Zhu, Lin Gu, Scott A. Chambers, Sujit Das, Timothy Charlton, Michael R. Fitzsimmons, Gang-Qin Liu, Shanmin Wang, Kui-juan Jin, Hongxin Yang, and Er-Jia Guo
Physical Review Lett. 128, 017202 (2022)
DOI: https://doi.org/10.1103/PhysRevLett.128.017202
23. Structural and Magnetic Properties of La0.7Sr0.3MnO3/LaCoO3 Heterostructures
S. Thota, K. Roychowdhury, V. Thakre, S. C. Ganguly, Z.H. Chen$, E J. Guo$, and S. Das$
Appl. Phys. Lett. 113, 122405 (2018)
DOI: https://doi.org/10.1063/1.5045359
24. Hexagonal close-packed polar-skyrmion lattice in ultrathin ferroelectric PbTiO3 films
Shuai Yuan, Zuhuang Chen, Sergei Prokhorenko, Yousra Nahas, Laurent Bellaiche, Chenhan Liu, Bin Xu, Lang Chen, Sujit Das, and Lane W. Martin
Physical Review Letters 130, 226801 (2023)
DOI: 10.1103/PhysRevLett.130.226801
25. Pure Chiral Polar Vortex Phase in PbTiO3/SrTiO3 Superlattices with Tunable Circular Dichroism
Sujit Das,* Margaret R. McCarter, Fernando G.mez-Ortiz, Yun-Long Tang, Zijian Hong, Anirban Ghosh, Padraic Shafer, Pablo Garc.a-Fern.ndez, Javier Junquera, Lane W. Martin, and Ramamoorthy Ramesh
Nano Letters (2023)
DOI: https://doi.org/10.1021/acs.nanolett.3c01744